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Chemical forms of γ-emitting radionuclides in soils adjacent to the Chernobyl NPP

Title: Chemical forms of γ-emitting radionuclides in soils adjacent to the Chernobyl NPP

Author: A.L. Kliashtorin, A.I. Shcheglov, F.A. Tikhomirov

Reference: Science of The Total Environment, Volume 164, Issue 3, 30 March 1995, Pages 177-184

DOI: http://dx.doi.org/10.1016/0048-9697(95)04464-C

Keywords: Radionuclides; Chernobyl NPP; Caesium; Soils

Abstract: Samples of sandy forest soils, meadow sandy-peat soil and meadow sandy-loam soil were taken at different sites within a 30-km zone around the Chernobyl NPP (ChNPP). The samples were extracted with water and a 0.1-N solution of ammonium acetate. The extracts were measured for γ-radionuclides and stable cation content. The content of all mobile forms of the radionuclides present in the 0–10-cm soil layer accounts for 0.5-5% of the total radionuclide content in this layer, depending on the type of radionuclide and soil. Water soluble forms of the radionuclides were found in the 0–5-cm layer only. Exchangable radionuclide forms were represented, as a rule, by radiocaesium in both the 0–5- and 5–10-cm layers. Content of Cs-137 exchangeable forms in the organic-mineral horizon were roughly inversely proportional to the sum of stable exchangeable cations and organic matter content. Forest vegetation takes up a significant share of the mobile forms of radiocaesium from the soils.

URL: http://www.sciencedirect.com/science/article/pii/004896979504464C

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