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VERTICAL MIGRATION OF RADIONUCLIDES IN THE VICINITY OF THE CHERNOBYL CONFINEMENT SHELTER

Title: VERTICAL MIGRATION OF RADIONUCLIDES IN THE VICINITY OF THE CHERNOBYL CONFINEMENT SHELTER

Author: Farfan, E. / Jannik, T. / Marra, J.

Reference: HEALTH PHYSICS JOURNAL, Oct 2011

Keywords: Chernobyl; radionuclide transport; fallout, migration

Abstract: Studies on vertical migration of Chernobyl-origin radionuclides in the 5-km zone of the Chernobyl Nuclear Power Plant (ChNPP) in the area of the Red Forest experimental site were completed. Measurements were made by gamma spectrometric methods using high purity germanium (HPGe) detectors with beryllium windows. Alpha-emitting isotopes of plutonium were determined by the measurement of the x-rays from their uranium progeny. The presence of {sup 60}Co, {sup 134,137}Cs, {sup 154,155}Eu, and {sup 241}Am in all soil layers down to a depth of 30 cm was observed. The presence of {sup 137}Cs and {sup 241}Am were noted in the area containing automorphous soils to a depth of 60 cm. In addition, the upper soil layers at the test site were found to contain {sup 243}Am and {sup 243}Cm. Over the past ten years, the {sup 241}Am/{sup 137}Cs ratio in soil at the experimental site has increased by a factor of 3.4, nearly twice as much as would be predicted based solely on radioactive decay. This may be due to ‘fresh’ fallout emanating from the ChNPP Confinement Shelter.

URL: http://www.osti.gov/bridge/product.biblio.jsp?query_id=2&page=0&osti_id=1024190

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